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adipate aggregation amino acid amylose average behaviour bonds branched calculated Chem chemical clots complex constant copolymer crosslinking curve cuticle cyclization decrease deformation density determined deuterated diluent dilution Dusek effect elastic modulus elastin elastomer entanglement equation equilibrium experimental experiments fibres fibrin fibrinogen Flory frame silk function galactomannan gel point gelatin gelation groups hydrodynamic radius increase inelastic loops interactions intramolecular intramolecular reaction kinetic length light scattering Macromolecules maltodextrin measurements mechanical melting molar molar mass molecular weight molecules monomer network chains network formation neutron scattering non-Gaussian non-linear observed obtained parameters PDMS Phys plot polybutadiene polyester polymer polymer networks polymerisation polymerization pre-gel predicted properties protein quaternary radius of gyration reacted relaxation resins ring samples segments shear modulus shown in Fig shows solution solvent spectra superspecies swelling degree swollen Table temperature theory uncrosslinked unsaturated values viscosity volume fraction