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A. N. Gent accelerator acid adhesion anionic Appl behavior block copolymers bond butadiene C. M. Roland carbon black chemical components composition concentration copolymerization cord crack crosslink crosslink density curing decrease deformation dependence devulcanization distribution dynamic effect elastic emulsion polymerization energy EPDM extruder FIGURE filler flow fracture free radical function graft graft copolymers groups hard segment hydrogen increase initiator internal mixer isoprene J. L. White Macromolecules materials measurements mixing modulus molecular weight molecules monomer morphology natural rubber obtained oxide particles peroxide phase Phys polybutadiene polyisoprene polymer chains Polymer Science polymerization polyurethanes ratio reaction reinforcement relaxation resistance result Rubber Chem rubber compounds sample shear shown in Fig silica soft segment solvent strain stress structure styrene sulfur surface tear Technol temperature tensile strength thermoplastic elastomers tion tire TPEs tread triblock U.S. Patent viscoelastic viscosity vulcanizates vulcanization York
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